The present invention relates to a multilayered polymeric body comprising multiple optical thickness layer types, at least a portion of which are in a folded relationship, which body reflects light and which can be fabricated to have an iridescent or silvery appearance; to decorative articles produced therefrom which may find use as wall panels, dishware, and decorative trims; and to security articles produced therefrom which may find use in anticounterfeiting applications.

The present invention provides a multilayered polymeric reflective body which can be iridescent or silvery in appearance, highly reflective, post formable, and capable of being fabricated into a variety of decorative and/or security articles The introduction of folded-over layers into the otherwise substantially planar layer structure of the body produces unique optical effects. The terms "reflective", "reflectivity", "reflection", and "reflectance" as used herein refer to total reflectance (that is, ratio of reflected wave energy to incident wave energy). For bodies which are silvery in appearance, the reflectance is sufficiently specular in nature such that the polymeric body has a metallic appearance. The use of these terms is intended to encompass semi-specular or diffuse reflection such as that of brushed metal and pewter.

A specific intensity of reflectance, when used herein, is the intensity of reflection which occurs at a wavelength where negligible absorption occurs. For example, a sil er appearing article reflects substantially all visible wavelengths (white light), whereas the introduction of a dye to achieve other metallic hues will necessarily lower reflectivity of the body at the absorbing wavelengths. Wavelengths unaffected by the dye will be reflected at essentially the same intensity as a non-dyed sample, and it is at these unaffected wavelengths to which the intensity of reflectance is referring. Likewise, where an article exhibits iridescent color, the intensity of reflection is measured at a wavelength corresponding to the color exhibited

According to one aspect of the present invention, a multilayer reflective polymeric Dody of at least first and second diverse polymeric materials is provided in wh,ch t* ^** e

first and second polymeric materials differ from each other in refractive index by at least about 0.03. The body should comprise a-suff icient number of alternating layers of the first and second polymeric materials such that at least a portion of the light incident on the body is reflected. As used herein, the term "light" is meantto encompass not only visible light but also electromagnetic radiation in both the infrared and ultraviolet regions of the spectrum. The term "a portion of the light incident on the body is reflected" refers, as discussed above, to reflected light at wavelengths where negligible absorption occurs.

At least a portion of the reflective polymeric body includes the alternating layers in a folded-over relationship which produces striations on portions on the body and results in a

10 number of optically unique, advantageous properties. The folded-over layers are formed while the body is in a freshly extruded condition. Excess material from several surface layers is caused to build up and then double over on itself causing a layer multiplication for that part of the body and producing the unique optical effects. Alternatively, the entire body may be caused to be folded upon itself. This folding can increase the number of layers in the body to double or

• _j 5 greaterthan the original number.

The portion of the body containing the folded-over layers has a greater reflectivity than the remaining portions of the body because of the presence of additional layers. Further, in one embodiment of the invention, addition of a coloring agent to one of the layers in the polymeric body imparts a three-dimensional appearance to the surface of the body

20 where the folded-over layers are located. The body is also versatile in its construction in that it may be constructed so as to appear silvery and/or iridescent in color, depending on the arrangement and optical thicknesses of the layers.

The optical thicknesses of the alternating layers may vary. In one embodiment of the invention, a substantial majority of the alternating layers have optical thicknesses of at

25 least 0.45 μm or less than 0.09 μm (optically thick or very thin layers, respectively). In an alternative embodiment, a portion of the alternating layers have optical thicknesses between 0.09 and 0.45 μm (optically thin), and the remaining layers have optical thicknesses of not greaterthan 0.09 μm or not less than 0.45 μm (optically thick very thin layers). In other embodiments of the invention, the alternating layers may all have optical thicknesses in the

30 range of from 0.09 μm to 0.45 μm. Thus, the polymeric body may comprise alternating optically thick layers, combinations of optically thick/very thin layers, combinations of optically thin and optically thick/very thin layers, or alternating optically thin layers.

Optically very thin layers (that is, less than 0.09 μm) as well as optically thick layers (that is, greaterthan 0.45 μm) reflect substantially white light over a wide spectrum of visible

35 wavelengths. Muftilayer bodies of alternating polymer iayers which are optically thick or a combination of optically thick and optically very thin possess a silvery, metallic appearance, while multilayer bodies comprising alternating polymer layers which are optically thi ^*** have an iridescent appearance with intense varying colors. The appearance of the body may be

controlled by the positioning and percentage of optically thin layers in the body. Further, in the practice of the present invention, the presence of folded-over layers adds a unique optical appearance to the surface of the body. The folded-over layers may comprise any of the three layer types described above. The reflective body of the present invention may be made up of two or more generally transparent polymer resins. Preferred are thermoplastic resins which are capable of being post formed into a variety of shapes. In a preferred embodiment of the invention, the first polymeric material comprises polycarbonate and the second polymeric material comprises polymethyl methacrylate. In other embodiments of the invention, elastomers may be used to provide a body which can be stretched and relaxed.

More than two different polymers may be present in the multilayer body. For example, the optically thin layers may comprise a pair of first and second polymers and the optically thick/very thin layers may comprise a pair of different first and second polymers. Folded-over layers may be introduced into either or both of the layer stacks. The layer types may then be laminated together as desired to form the reflective body.

The reflective polymeric body is preferably in the form of a sheet having two major exterior surfaces. An outer layer may be included as a surface or skin layer on both major exterior surfaces of the reflective body. The skin layer may be sacrificial, or may be permanent and serve as a scratch resistant and weatherable protective layer. The skin layer is preferably applied to the bodyduring or after extrusion of the multilayer construction. For example, a skin layer may be applied as a sprayed on coating which acts to level the surface of the body to improve optical properties and impart scratch resistance, chemical resistance and/or weatherability. The skin layer may also be laminated to the multilayered body.

In certain embodiments of the invention, to obtain high reflectivity it is desirable . to form the reflective polymeric body to comprise at least 500 or more layers. Increasing the total number of layers in the polymeric body has been found to increase its reflectivity (that is, the percentage of incident light reflected from the body). Thus, by controlling the number of layers, the degree of reflectivity of the article may be controlled. Areas of the body having folded-over layers will exhibit greater reflectivity because of the presence of additional layers in that portion of the body.

The multilayer reflective polymeric bodies of the present invention may be post formed into a number of decorative or useful items. Such post forming operations may include thermoforming, vacuum forming, or pressure forming. Further, through the use of forming dies, the multilayer reflective body may be initially formed into a variety of useful shapes including profiles such as bodies having angled portions, flanges and T-shapes. The multilayer reflective polymeric bodies of the present invention may also find uses in security applications such as on currency or as credit card emblems as indicia of authenticity or as devices which

cannot be readily reproduced or copied by counterfeiters. The multilayer reflective bodies may also be formed into the credit card substrate itself.

The present invention provides an extrusion apparatus for preparation of the multilayer reflective body of the present invention comprising at least first and second sources of heat plastified thermoplastic material, and combining means for receiving the heat plastified material from the first and second sources and arranging the first and second sources of heatplastified materials in a layered relationship to form a composite stream. A shaping die in communication with the combining means is also provided which is arranged so as to permit substantially streamlined flow of the composite stream through the die to form the multilayer body- Means are also included adjacent the shaping die for modifying at least the surface of at least a portion of the multilayer body to fold over at least some of the layers onto themselves. Such means includes at least two cooling rolls positioned on opposing sides of the multilayer body exiting the die. A means for driving the cooling rolls is also provided wherein the cooling rolls are operated at a slower speed than the speed of the multilayer body exiting the die (or material from the die is supplied at a faster rate than the speed of operation of the rolls), causing an excess of layered material on the intake side of the rolls to be built up and folded over as the multilayer body passes between the rolls. The speed of the rolls may be cyclically varied to create and maintain the folding of the layers on a substantially continuous basis. Alternatively, the apparatus may be controlled to cause the entire body to fold over upon itself. Lateral fold over in the machine direction may also be promoted by extruding a sheet having a non-uniform surface using a die having serrated or sawtooth shaped die lips.

The present invention also provides a method for preparing a multilayer reflective polymeric body comprising the steps of providing at least first and second streams of heatplastified thermoplastic materials, receiving and combining the first and second streams of materials in a layered relationship to form a composite stream, directing the composite stream to flow through a shaping die to form a multilayer body, and modifying at least the surface of at least a portion of the multilayer body by folding over a portion of the layers onto themselves. Alternatively, the entire body may be caused to fold over upon itself. A preferred method of modifying at least the surface of the multilayer body includes the step of passing the multilayer body through at least two cooling rolls positioned on opposing sides of the body. The cooling rolls are operated so that an excess of layered material on the intake side of the rolls is built up and then flattened onto the surface of the sheet as the sheet passes between the rolls to form folded-over layers on the multilayer body. Preferably, the cooling rolls are operated at a slower linearspeed than the speed of the multilayer body exiting the die. Alternatively, the amount of multilayer material exiting the die ma be increased. In addition, the speed of the cooling rolls is preferably cyclically varied so asto create and maintain the folding of the layers on a substantially continuous basis.

Accordingly, it is an object of the present invention to provide a multilayer reflective polymeric body having unique optical properties comprising multiple optical thickness layer types which have folded-over layers on at least a portion of the surface of the body and which can be fabricated into a variety of decorative and security articles, is post formable, and which may have an iridescent or colorless appearance. This, and other objects and advantages of the invention will become apparent from the following detailed description, the accompanying drawings, and the appended claims.

Fig. 1 is a schematic representation of an apparatus for preparing the multilayered polymeric body of the present invention; Fig- 2 is an expanded schematic view illustrating the cooling rolls of the extrusion apparatus of the present invention and the bank of thermoplastic material which is caused to accumulate at the intake side of the rolls;

Fig. 3 is a side view of the structure of the multilayer reflecti e polymeric body of the present invention showing folded-over layers; Figs. 4A and 4B are perspective views of the multilayer reflective polymeric body of the present invention showing non-uniform extruded surfaces, wavy in Fig. 4A and saw- toothed in Fig.4B, to encouraged layer fold over in the machine direction; and

Figs. 5A and 5B are sectional views of the bodies of Figs.4A and B, respectively, after a portion of the layers have been folded over. The present invention provides a highly reflective multilayer polymeric body made up of from a hundred to several thousand layers of the same or different types of optical layers. The alternating layers of polymeric materials may have an optical thickness of at least 0.45 μm (optically thick), or may have a combination of optically thick layers with layers having an optical thickness of not greater than 0.09 μm (optically very thin), or may have optical thicknesses between 0.09 and 0.45 μm (optically thin), where the optical thickness is defined as the product of the individual layer thickness times the refractive index of the polymeric material which makes up that layer. Different combinations of layertypes will produce a reflective body having different appearances. Likewise, the optical thicknesses of the folded- over layers or striated layers will affect the appearance of the body giving the surface of the body a three-dimensional appearance. The thicknesses of the individual layers may be controlled to some extent by the layer forming and manipulation steps explained in greater detail below. Generally, as the layers are folded over, a thinning of individual layer thicknesses occurs.

Thus, in one form of the invention, the polymeric reflective body comprises either optically thick layers of at least 0.45 μm, or combinations of optically thin layers and optically thick and/or very thin layers having optical thicknesses of not greater than 0.09 μm or not less than 0.45 μm, respectively, to produce a silvery reflective appearance The use of a substantial number of optically thin layers in the body produces vivid, iridescent reflected colors.

For purposes of optical properties, that is, reflectance and transmittance, an optically thin layer can be described as a layer having an optical thickness in the range of from λ/4to 5 λ/4, where λ represents the visible wavelength range. Thus, for layers to be used in the visible wavelength band, an optically thin layer has been described in the literature as one whose thickness, D, is less than 0.5 μm or whose optical thickness, ND (where N is the refractive index of the material) is less than 0.7 μm. Vasicek, Optics of Thin Films (1960) at pages 100 and 139.

Opticallythin film layers rely on the constructive optical interference of light to produce intense reflected light in the visible, ultraviolet, or infrared portions of the electromagnetic spectrum accordingto the equation (for a two component system): λ _m = (2/m) (N ₁ D ₁ + N ₂ D ₂ ), where λ _m is the reflected wavelength in nanometers, Nt and N ₂ are the refractive indices of the alternating polymers, Di and D are the thickness of the respective layers of polymers in nanometers, and m is the order of reflection (m = 1 ,2,3,4,5). Each solution of the equation determines a wavelength at which an intense reflection, relative to surrounding regions, is expected. The intensity of the reflection is a function of the "f-ratio" where, f S NT D^NT D, + N ₂ D ₂ ) .

By proper selection of the f-ratio, one can exercise some degree of control over the intensity of reflection of the various higher order reflections. For example, first order visible reflections of violet (0.38 μm wavelength) to red (0.68 μm wavelength) can be obtained with layer optical thicknesses between 0.075 to 0.25 μm. Iridescent films may also be designed to reflect visible light at higher order reflectances, although at lower intensities.

For certain embodiments of the invention, it is desirableto use opticallythin layers in combination with optically thick layers or combinations of optically thick/very thin layers sothatthe reflective body will exhibit a colored or silvery iridescence. The opticallythin layers ma be in the folded-over layers or may be in the remainder of the body.

In other embodiments of the invention, the multilayer bodies are designed so that they do not display vivid iridescence. By combining layers which are too thick or too thin to cause iridescence, a reflection which is essentially silver and non-iridescent results. This silvery appearance is due to higher order reflections from the optically thick and/or very thin layers being so closely spaced that the human eye perceives the reflection to be essentially non- iridescent.

For a two component system of alternating layers of polymers having optical thicknesses in the thick or very thin range, the reflective characteristics of articles are governed by the following equation:

R = (kr)/(1 + (k - 1)r) x 100,

where R is the amount of reflected light (%), k is the sum of optically thick and optically thick/very thin layer interfaces, and r = [(Nι - N ₂ )/(Nι + N ₂ )p. See Vasicek. Optics of Thin Films (1960) at pages 69-70.

This equation indicates that the intensity of the reflected light is a function only of r and k, where r and k are defined as above. As a close approximation, R is a function only of the refractive index mismatch of the two polymer components and the number of layer interfaces.

The present invention judiciously combines layers having differing optical thicknesses to obtain a multilayer reflective polymeric body which exhibits a unique iridescent o or colorless reflectance, depending upon the desired combination of layers. By positioning the folded-over layers at different portions of the surface of the body, additional unique optical effects are provided.

The reflective polymeric bodies of the present invention become more highly reflective of incident light (that is, transmit less light) as the number of layers is increased. 5 Preferably, the number of layers is sufficient to produce an article which will reflect at least 30 percent of the incident light for those wavelengths for which there is negligible absorption. Reflectances below about 30 percent are not sufficient to be readily observed except for iridescence.

The reflectivity of the body is affected by the difference in refractive index 0 between the various polymers making up the reflective body. That is, the greater the difference in refractive index at each layer interface, the greater the reflectivity of the body Accordingly, it can be seen that the reflective nature of the polymeric bodies may be controlled by the selection of polymers.

The reflective multilayered polymeric bodies of the present invention may 5 comprise alternating layers of a wide variety of generally transparent thermoplastic materials. Suitable thermoplastic resins, along with representative refractive indices, which may be used in the practice of the present invention include, but are not limited to: copolycarbonates of bisphenol and thiodiphenol (refractive index = 1.59 to 1.64), blends of polymethyl methacrylate and polyvinylidene fluoride (1.38 to 1.49), bisphenol A polycarbonate (1.59), 0 copolymers of methyl methacrylate and vinylidene fluoride (1.42 to 1.38), polymethyl acrylate (1.48), polymethyl methacrylate (1.49), blends and copolymers of polymethyl methacrylate and polyvinylidene fluoride; copolymers of vinylidene fluoride and other halogenated monomers such as chlorofluoroethylene, chlorodifluoroethylene, chlorotrifluoroethylene, hexafluoroacetone, hexafluoropropylene, hexafiuoropropene, pentafiuoropropylene, 5 trifluoroethylene, tetrafluoroethylene, and vinyl fluoride blended with polymethyl methacrylate; blends of polyvinylidene fluoride and poly(vinyl acetate), copolymers of methyl methacrylate, vinylidene fluoride, and a monomer selected from the group consisting of chlorofluoroethylene, chlorodifluoroethylene, chlorotrifluoroethylene, hexafluoroacetone,

hexafluoropropylene, hexafluoropropene, pentafluoropropylene, trifluoroethylene, tetrafluoroethylene,and vinyl fluoride blended with polymethyl methacrylate; blends of polyvinylidene fluoride and poly(vinyl acetate); perfluoroalkoxy resins (1.35); polytetrafluoroethylene (1.35); fluorinated ethylene-propylene copolymers (1.34); silicone resins (1.41); polyvinylidene fluoride (1.42); polychlorotrifluoroethylene (1.42); epoxy resins (1.45); poly(butyl acrylate) (1.46); poly(4-methylpentene-1) (1.46), poly(vinyl acetate) (1.47), ethyl cellulose (1.47), polyformaldehyde (1.48), polyisobutyl methacrylate (1.48), polymethyl acrylate (1.48), polypropyl methacrylate (1.48), polyethyl methacrylate (1.48), polyether block amide (1.49); cellulose acetate (1.49); cellulose propionate (1.49); cellulose acetate butyrate (1-49), cellulose nitrate (1.49), polyvinyl butyral (1.49), propylene (1.49); polybutylene (1.50); ionomeric resins such as Suriyn (trademark) (1.51 ), low density polyethylene (1.51), polyacrylonitrile (1.51), polyisobutylene (1.51), thermoplastic polyesters such as Ecdel (trademark) (1.52); natural rubber (1.52); perbunan (1.52); polybutadiene (1.52); nylon (1.53); poiyacrylic imides (1.53); poly(vinyi chloro acetate) (1.54); polyvinyl chloride (1.54); high density polyethylene (1.54); copolymers of methyl methacrylate and styrene such as Zerlon (trademark) (1.54); transparent acrylonitrile-butadiene-styreneterpolymer (1.54); allyl diglycol resin (1.55), blends of polyvinylidene chloride and polyvinyl chloride such as Saran resins (trademark) (1.55); polyalpha-methyl styrene (1.56); styrene-butadiene latexes such as Dow 512-. (trademark) (1.56), polyurethane (1.56); neoprene (1.56); copolymers of styrene and acrylonitrile such as Tyril resin (trademark) (1.57); copolymers of styrene and butadiene (1.57); polycarbonate (1.59); other thermoplastic polyesters such as polyethylene terephthalate and polyethylene terephtha I ate glycol (1.60); polystyrene (1.60); polyimide (1.61); polyvinylidene chloride (1.61 ); polydichlorostyrene (1.62); pofysulfone (1.63); polyether sulfone (1.65); and polyetherimide (1.66). A condition for the selection of the polymers to make up the layers of the body is that the pofymers selected have refractive indices which differ from each other by at least about 0.03. Further, the polymers should preferably be compatible in processing temperatures so that they may be readily coextruded.

Atypical extrusion apparatus for the preparation of the multilayer reflective body of the present invention is illustrated schematically in Fig. 1. There, extrusion apparatus 10 includes, in cooperative combination, first, second, and optional third sources of heat plastif ied polymeric resins for extruders 1 1, 12, and 13, respectively. An Optional third source of polymer resin may used when it is desired to produce a body having different layer repeating unit patterns such as ABCABC or ABCBABCB or when it is desired to provide protective boundary layers with the body. The third polymer may differ in refractive index from the first and second polymers. In one embodiment, the third polymer may comprise a copolymer of the first and second components.

Extruders 11 , 12, and (optionally) 13 discharge the heat plastified polymeric resins into conduits 14, 15, and 16, respectively. A coextrusion feedblock die 17 is in operative combination with conduits 14, 15, and 16 and receives first, second, and optional third heat plastified streams therefrom. A heat plastified polymer stream may also be fed into the upstream end of feedblock die 17 to form protective boundary layers as the polymers are coextruded. Die 17 combines and arranges the heat plastified polymers into layered relationships as taught in U.S. Patent Nos. 3,773,882 and 3,884,606. Die 17 further defines an extrusion orifice 18 from which issues a composite stream of polymeric material having alternating substantially planar layers of first and second (and optionally third) polymeric materials.

From orifice 18, the composite stream passes optionally through a mechanical manipulating section 20 which serves to rearrange the alternating layers into a stream having more than the original number of layers as taught in the aforementioned U.S. Patent Nos. 3,565,985 and 3,759,647. Additional manipulating sections may be arranged in series to further multiply the number of layers in the stream. The number of additional layers created using the manipulation devices of the aforementioned patents is determined by the number of layers divided by the layer-dividing vane in those devices.

The multilayered stream is then passed into a shaping die 22 which is so constructed and arranged that streamlined flow is maintained therein. Such an extrusion die is described in U.S. Patent No. 3,557,265, the disclosure of which is incorporated by reference herein. While a sheet orfilm forming die 22 is illustrated, it will be appreciated by those skilled in the art that a forming die of any desired configuration may be used to extrude not only films and sheets, but also other profiles and shapes. Further, the lips of the die may be serrated, saw- toothed, or wavy in configuration to provide non-uniformities 42 in the surface of the extruded body 44 as illustrated in Figs. 4A (sinusoidal waves) and 4B (saw-tooth ridges). These surface non-uniformities promote the folding over of the layers in the machine direction of travel of the body as described in greater detail below.

The configuration of the shaping die can vary and can be such as to reduce the thickness of each of the layers. The precise degree of reduction in thickness of the layers delivered from the mechanical orienting section, the configuration of the die, and the amount of mechanical working of the body after extrusion are all factors which affect the thickness of the individual layers in the final body.

Means are also included adjacent the shaping die for modifying at least the surface of at least a portion of the multilayer body to fold over at least some of the layers onto themselves. As illustrated in Fig. 2, such means comprise two cooling rolls 30, 31 positioned on opposing sides of the multilayer body 32 exiting the die. A means for driving the cooling rolls is also provided in which at least one of the cooling rolls is operated at a slower speed than the speed of the multilayer body exiting the die, causing an excess of layered material 34 on the

intake side of the rolls to be built up and folded over as the multilayer body passes between the rolls. Depending on the relative speeds of rolls 30, 31 and the orientation of the body, excess ^■ material may be built up on one or both surfaces of the body. Fig. 3 illustrates the alternating layers 36 as they appear in the final sheet of the polymeric reflective body. As is shown, layers 40 are in a folded-over relationship which increase the total numbers of layers in that portion of the body.

It must be remembered that the multilayer bodies of the present invention may comprise up to several hundred or a thousand or more layers having thicknesses of only a fraction of a micrometer. Thus, illustration of the layers in the drawings, both as to number and thickness, is greatly simplified and exaggerated for ease of understanding.

Thus, in the embodiment illustrated in Fig. 2, the excess material is built up and flattened on the surface of the sheet to form folded-over layers on the final multilayer body. This produces layer fold over in a direction generally normal to the direction of travel of the sheet (machine direction). In order to maintain the proper layer multiplication on a continuous basis, the speed of the cooling rolls is preferably cyclically varied. As an example, the speed of the cooling rolls may be cyclically varied between about 1 ft/min and 5 ft/mϊn. Where the layered body is extruded downwardly in a vertical direction between cooling rolls 30, 31 , a bank of excess material may be caused to build up on both surfaces of the body.

In another embodiment of the invention, one or both of the die lips on forming die 22 may have a serrated, saw-toothed, or wavy configuration to produce non-uniformities 42 in one or both surfaces of the extruded bodies. These non-uniformities promote lateral fold over of the layers as shown in Figs. 5A and 5B. As the sheet or body passes between cooling rolls 30, 31, the layered polymeric material in areas 46 (best seen in Figs. 5Aand 5B) flows and folds into the areas of non-uniformity. Reflective polymeric bodies produced by the practice of the present invention have a wide variety of useful applications. In some embodiments of the invention it may be desirable to incorporate coloring agents such as dyes or pigments into one or more of the individual layers of the polymeric body. It is desirable to use pigmented coloring agents in the interior layers to impart a three-dimensional appearance to the surface of the body. This can be done to one of the outer or ski n layers of the body, or alternatively, the colori ng agent may be incorporated into one or more interior layers in the body. The coloring agents may be selected to give the polymeric body a metallic appearance other than its normal silvery appearance such as bronze, copper, or gold, for example.

Different colors such as black, blue, red, yellow and white may also be used Coloring agents ma be used in combination to provide desirable coloring and optical properties.

Additionally, the highly reflective polymeric bodies may be fabricated as non- corroding metallic appearing articles for indoor or outdoor exposure. For example, the

polymeric bodies may be fabricated into signs, or bright work for appliances. The bodies may be ^" post formed into highly reflective decorative items such as wall panels, dishware and decorative trims, by processes such asthermoforming, vacuum forming, shaping, rolling, or pressure forming. The bodies may also be used for security applications such as credit card emblems or on currency. For example, the body may be embedded into or secured onto the surface of a credit card similar to the manner in which holographic or prismatic foils are currently used. Alternatively, the body may be formed into the credit card itself. The body may also be secured to a portion of a document, such as a document indicating title. The body may also be used on o paper currency, or be formed into plastic currency. in order that the invention may be more readily understood, reference is made to the following example, which is intended to be illustrative of the invention, but is not intended to be limiting in scope. Example 1 5 A 2,625 layer melt stream of CALIBRE 303-22 (trademark) polycarbonate

(refractive index 1.59) and Acrylite H15-003 (trademark) polymethyl methacrylate (refractive index 1.49) was produced using a 165 layer feedblock and four layer multipliers as taught in U.S. Patent Nos.3,773,882 and 3,759,647. In addition, skin layers were extruded onto both exterior surfaces of the melt stream which comprised 75 percent by weight CALIBRE 303-22 0 (trademark) polycarbonate and 25 percent by weight polycarbonate dye concentrate. Roll speed was cycled manually between 1 ft/min and 5 ft/min in order to continually produce folded-over layers in the body like those illustrated in Figs. 2 and 3. The multilayer sheet which was produced had an overall silvery reflective appearance with areas of varying intense iridescent color indicating the presence of both optically thick and/or optically very thin layers 5 as well as optically thin layers. The folded-over layers exhibited a three-dimensional stepped visual effect of overlapping stacked layers similar to a deck of cards where the cards are offset from adjacent cards in the deck.

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